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Pods does not offer this kind of functionality at the moment. You can make any single field repeatable but that’s just one field. Like a list of names. Or a list of phone numbers. But not rows with multiple fields that repeat.
What you may want to look at is our Flexible Relationships feature:
That video goes through how it works, but essentially it allows you to enter as many values as you want and they use relationships to store the information on their own separate content type. In your case, you could have a “Contact” post type there.